Abstract
Nucleonic matter displays a quantum-liquid structure, but in some cases finite nuclei behave like molecules composed of clusters of protons and neutrons. Clustering is a recurrent feature in light nuclei, from beryllium to nickel1,2,3. Cluster structures are typically observed as excited states close to the corresponding decay threshold; the origin of this phenomenon lies in the effective nuclear interaction, but the detailed mechanism of clustering in nuclei has not yet been fully understood. Here we use the theoretical framework of energy-density functionals4,5, encompassing both cluster and quantum liquid-drop aspects of nuclei, to show that conditions for cluster formation can in part be traced back to the depth of the confining nuclear potential. For the illustrative example of neon-20, we show that the depth of the potential determines the energy spacings between single-nucleon orbitals in deformed nuclei, the localization of the corresponding wavefunctions and, therefore, the degree of nucleonic density clustering. Relativistic functionals, in particular, are characterized by deep single-nucleon potentials. When compared to non-relativistic functionals that yield similar ground-state properties (binding energy, deformation, radii), they predict the occurrence of much more pronounced cluster structures. More generally, clustering is considered as a transitional phenomenon between crystalline and quantum-liquid phases of fermionic systems.
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References
Weizsäcker, C. F. V. Neuere Modellvorstellungen über den Bau der Atomkerne. Naturwissenschaften 26, 209â217 (1938)
Wheeler, J. A. On the mathematical description of light nuclei by the method of resonating group structure. Phys. Rev. 52, 1107â1122 (1937)
Von Oertzen, W. V., Freer, M. & Kanada-Enâyo, Y. Nuclear clusters and nuclear molecules. Phys. Rep. 432, 43â113 (2006)
Bender, M., Heenen, P.-H. & Reinhard, P.-G. Self-consistent mean-field models for nuclear structure. Rev. Mod. Phys. 75, 121â180 (2003)
Vretenar, D., Afanasjev, A. V., Lalazissis, G. A. & Ring, P. Relativistic HartreeâBogoliubov theory: static and dynamic aspects of exotic nuclear structure. Phys. Rep. 409, 101â259 (2005)
Kanada-Enâyo, Y. & Horiuchi, H. Structure of light unstable nuclei studied with antisymmetrized molecular dynamics. Prog. Theor. Phys. 142 (Suppl.). 205â263 (2001)
Feldmeier, H., Bieler, K. & Schnack, J. Fermionic molecular dynamics for ground states and collision of nuclei. Nucl. Phys. A 586, 493â532 (1995)
Neff, T. & Feldmeier, H. Tensor correlations in the unitary correlation operator method. Nucl. Phys. A 713, 311â371 (2003)
Tohsaki, A., Horiuchi, H., Schuck, P. & Röpke, G. Alpha cluster condensation in 12C and 16O. Phys. Rev. Lett. 87, 192501 (2001)
Fynbo, H. O. U. et al. Revised rates for the stellar triple-α process from measurement of 12C nuclear resonances. Nature 433, 136â139 (2005)
Rose, H. J. & Jones, G. A. A new kind of natural radioactivity. Nature 307, 245â247 (1984)
Greiner, W., Park, J. Y. & Scheid, W. Nuclear Molecules (World Scientific, 1995)
Ikeda K, Tagikawa N & Horiuchi H The systematic structure-change into the molecule-like structures in the self-conjugate 4n nuclei. Prog. Theor. Phys. 464 (Suppl.). 464â475 (1968)
Arumugam, P., Sharma, B. K. & Patra, S. K. Relativistic mean field study of clustering in light nuclei. Phys. Rev. C 71, 064308 (2005)
Maruhn, J. A. et al. α-Cluster structure and exotic states in a self-consistent model for light nuclei. Phys. Rev. C 74, 044311 (2006)
Reinhard, P.-G., Maruhn, J. A., Umar, A. S. & Oberacker, V. E. Localization in light nuclei. Phys. Rev. C 83, 034312 (2011)
Okolowicz, J., Ploszajczak, M. & Nazarewicz, W. On the origin of nuclear clustering. Preprint at ãhttp://arxiv.org/abs/1202.6290ã (2012)
Girod, M. & Grammaticos, B. Triaxial HartreeâFockâBogolyubov calculations with D1 effective interaction. Phys. Rev. C 27, 2317â2339 (1983)
Ichikawa, T., Marhun, J. A., Itagaki, N. & Ohkubo, S. Linear chain structure of four-α clusters in 16O. Phys. Rev. Lett. 107, 112501 (2011)
Robledo, L. M. & Bertsch, G. F. Global systematics of octupole excitations in evenâeven nuclei. Phys. Rev. C 84, 054302 (2011)
Chabanat, E., Bonche, P., Haensel, P., Meyer, J. & Schaeffer, R. A Skyrme parametrization from subnuclear to neutron star densities part II. Nuclei far from stabilities. Nucl. Phys. A 635, 231â256 (1998)
Lalazissis, G. A., NikÅ¡iÄ, T., Vretenar, D. & Ring, P. New relativistic mean-field interaction with density-dependent meson-nucleons couplings. Phys. Rev. C 71, 024312 (2005)
Fricke, G. et al. Behavior of the nuclear charge radii systematics in the s-d shell from muonic atom measurement. Phys. Rev. C 45, 80â89 (1992)
Chulkov, L. et al. Interaction cross sections and matter radii of A = 20 isobars. Nucl. Phys. A 603, 219â237 (1996)
Nilsson, S. G. Binding states of individual nucleons in strongly deformed nuclei Mat. Fys. Medd. Dan. Vid. Selsk. 29, 1â69 (1955)
Cohen-Tannoudji, C., Diu, B. & Laloë, F. Mécanique Quantique (Hermann Ed., 1973)
Walecka, J. D. Theoretical Nuclear and Subnuclear Physics (Imperial College Press and World Scientific, 2004)
Mottelson, B. Elementary features of nuclear structure. In Les Houches Session LXVI, Trends in Nuclear Physics, 100 Years Later (eds Nifenecker, H., Blaizot, J.-P., Bertsch, G. F., Weise, W. & David, F. ). 25â121 (North-Holland Elsevier, 1996)
Pines, D. & Nozières, P. The theory of quantum liquids (Benjamin, 1966)
Stoitsov, M. V., Dobaczewski, J., Nazarewicz, W. & Ring, P. Axially deformed solution of the SkyrmeâHartreeâFockâBogolyubov equations using the transformed harmonic oscillator basis. The program HFBTHO (v1.66p). Comput. Phys. Commun. 167, 43â63 (2005)
Acknowledgements
This work was supported by the Institut Universitaire de France and by the Croatian Ministry of Science, Education and Sportâproject 1191005-1010. The authors thank J. Margueron, M. Milin, T. Neff, N. Van Giai and P. Schuck for comments and suggestions.
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Model calculations were done by J.-P.E., E.K., T.N. and D.V. The manuscript text was prepared by E.K. and D.V. with contributions from J.-P.E. and T.N. J.-P.E. and E.K. prepared the figures.
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Ebran, JP., Khan, E., NikÅ¡iÄ, T. et al. How atomic nuclei cluster. Nature 487, 341â344 (2012). https://doi.org/10.1038/nature11246
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DOI: https://doi.org/10.1038/nature11246